An Efficient Turing‐Type Ag <sub>2</sub> Se‐CoSe <sub>2</sub> Multi‐Interfacial Oxygen‐Evolving Electrocatalyst**
نویسندگان
چکیده
Although the Turing structures, or stationary reaction-diffusion patterns, have received increasing attention in biology and chemistry, making such unusual patterns on inorganic solids is fundamentally challenging. We report a simple cation exchange approach to produce Turing-type Ag2Se CoSe2 nanobelts relied diffusion-driven instability. The resultant Ag2Se-CoSe2 material highly effective catalyze oxygen evolution reaction (OER) alkaline electrolytes with an 84.5 % anodic energy efficiency. Electrochemical measurements show that intrinsic OER activity correlates linearly length of interfaces, determining interfaces are more active sites for OER. Combing X-ray absorption computational simulations, we ascribe excellent performance optimized adsorption energies critical oxygen-containing intermediates at unconventional interfaces.
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ژورنال
عنوان ژورنال: Angewandte Chemie
سال: 2021
ISSN: ['1521-3773', '1433-7851', '0570-0833']
DOI: https://doi.org/10.1002/anie.202017016